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However, issues of rapid charge recombination of these photoelectrochemical storage materials and misaligned band energy of the devices have resulted in a limited efficiency that hampers the development of coupled solar batteries. In contrast, the emerging coupled solar batteries allow direct solar energy storage via a photo-coupled ion transfer at photoelectrochemical storage electrode materials with both light harvesting and redox activity. Integrated solar batteries that integrate photoelectrodes with redox-electrodes realize indirect solar energy storage based on dual energy matching (photo-carriers and redox couples) and two distinct processes (electricity generation and redox reaction). Solar-to-electrochemical energy storage in solar batteries is an important solar utilization technology alongside solar-to-electricity (solar cell) and solar-to-fuel (photocatalysis cell) conversion.
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